Wheel-like Gd<sub>42</sub> polynuclear complexes with significant magnetocaloric effect

نویسندگان

چکیده

Two 42-nuclearity lanthanide complexes with a wheel-like structure were synthesized, in which Gd congeners exhibited significant magnetocaloric effect due to the high isotropy nuclearity and weak ferromagnetic interactions.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Polynuclear Gold(I) Complexes of Mercaptocarboxylic Acids

Gold(I) Thiolates, (Benzylthiolato)gold(I) Complexes, Gold(I) Mercaptocarboxylates, Polynu­ clear Gold(I) Complexes In a search for air-stable and water-soluble mercapto compounds of gold with a high gold content, benzylthiol, a-mercapto-acetic acid, /3-mercapto-propionic acid, and thiosalicylic acid were converted into aurated sulfonium salts by treatment with reagents of the type [(R^PjAufiO*...

متن کامل

Polynuclear palladium complexes with biogenic polyamines: AFM and voltammetric characterization.

Polynuclear Pd(II) complexes with biogenic polyamines present great potential clinical importance, due to their antiproliferative and cytotoxic activity coupled to less severe side-effects. The adsorption process and the redox behaviour of two polynuclear palladium chelates with spermine (Spm) and spermidine (Spd), Pd(II)-Spm and Pd(II)-Spd, as well as of their ligands Spm and Spd, were studied...

متن کامل

Magnetocaloric effect in La0.75Sr0.25MnO3 manganite

The polycrystalline manganite La0.75Sr0.25MnO3 prepared by an alternative carbonate precipitation route reveals the rhombohedral perovskite structure. Magnetization isotherms measured up to 2 T are used to determine Curie temperature of 332 K by means of Arrott plot. Maximum of magnetic entropy change is found at Curie temperature. The relative cooling power equal to 64 J/kg for 1.5 T magnetic ...

متن کامل

Multiple magnetic relaxation processes, magnetocaloric effect and fluorescence properties of rhombus-shaped tetranuclear rare earth complexes.

Seven new tetranuclear rare earth (RE) complexes [RE4(acac)4L6(μ3-OH)2] (HL = 5-(4-fluorobenzylidene)-8-hydroxylquinoline; acac = acetylacetonate; RE = Y (1), Eu (2), Gd (3), Tb (4), Dy (5), Tm (6) and Lu (7)) have been synthesized and completely characterized. Complex exhibits multiple zero-field slow magnetic relaxation processes typical of Single Molecule Magnets (SMMs). Two distinct slow ma...

متن کامل

Polynuclear lanthanide hydroxo complexes: new chemical precursors for coordination polymers.

The synthesis of hexanuclear lanthanide hydroxo complexes by controlled hydrolysis led to polymorphic compounds. The hexanuclear entities crystallize in four different ways that depend on the extent of their hydration. The four structures can be described as hexanuclear lanthanide entities with formula [Ln(6)(mu(6)-O)(mu(3)-OH)(8)(NO(3))(6)(H(2)O)(12)](2+). Two additional NO(3)(-) ions intercal...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: CrystEngComm

سال: 2022

ISSN: ['1466-8033']

DOI: https://doi.org/10.1039/d2ce00315e